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Improved and General Manganese-Catalyzed N-Methylation of Aromatic Amines Using Methanol

Abstract : A novel lutidine-based manganese PNP-pincer complex has been synthesized for the selective N-methylation of aromatic amines with methanol. Using borrowing hydrogen methodology, a selection of differently functionalized aniline derivatives is selectively methylated in good yields.
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https://hal-univ-rennes1.archives-ouvertes.fr/hal-01518033
Contributor : Laurent Jonchère <>
Submitted on : Thursday, May 4, 2017 - 10:31:08 AM
Last modification on : Saturday, July 11, 2020 - 3:16:47 AM

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Jacob Neumann, Saravanakumar Elangovan, Anke Spannenberg, Kathrin Junge, Matthias Beller. Improved and General Manganese-Catalyzed N-Methylation of Aromatic Amines Using Methanol. Chemistry - A European Journal, Wiley-VCH Verlag, 2017, 23 (23), pp.5410-5413. ⟨10.1002/chem.201605218⟩. ⟨hal-01518033⟩

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