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Synthesis of metathesis catalysts with fluorinated unsymmetrical N,N’-diaryl imidazoline-based NHC ligands

Abstract : New olefin metathesis catalysts bearing unsymmetrical fluorinated NHC ligands with hexafluoroisopropylmethoxy group in ortho-positions of N-aryl-substituent have been synthesized. The effects of mono-ortho-arylsubstitution and the replacement of para-methyl N-aryl group with more electron-donating methoxy group in unsymmetrical fluorinated NHC ligand on the activity of complexes have been evaluated.
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Submitted on : Monday, September 4, 2017 - 2:38:34 PM
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S.M. Masoud, M.A. Topchiy, A.S. Peregudov, T. Roisnel, P.H. Dixneuf, et al.. Synthesis of metathesis catalysts with fluorinated unsymmetrical N,N’-diaryl imidazoline-based NHC ligands. Journal of Fluorine Chemistry, Elsevier, 2017, 200, pp.66-76. ⟨10.1016/j.jfluchem.2017.06.004⟩. ⟨hal-01581217⟩

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