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Iridium Catalyzed Hydrogenation and Dehydrogenation of N-Heterocycles in Water under Mild Conditions

Abstract : An efficient catalytic method is presented for the hydrogenation of N-heterocycles. The iridium-based catalyst operates under mild conditions in water without any co-catalyst or stoichiometric additives. The catalyst also promotes the reverse reaction of dehydrogenation of N-heterocycles, hence displaying appropriate characteristics for a future hydrogen economy based on liquid organic hydrogen carriers (LOHCs).
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https://hal-univ-rennes1.archives-ouvertes.fr/hal-02087810
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Submitted on : Thursday, July 18, 2019 - 11:43:22 AM
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Shengdong Wang, Haiyun Huang, Christian Bruneau, Cedric Fischmeister. Iridium Catalyzed Hydrogenation and Dehydrogenation of N-Heterocycles in Water under Mild Conditions. ChemSusChem, ChemPubSoc Europe/Wiley, 2019, 12 (11), pp.2350-2354. ⟨10.1002/cssc.201900626⟩. ⟨hal-02087810v2⟩

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